TY - JOUR
T1 - Evaluated and recommended cross section data for production of radionuclides with emerging interest in nuclear medicine imaging. Part 2 : Single photon emission computed tomography (SPECT)
AU - Hermanne, Alex
AU - Tarkanyi, Ferenc
AU - Ignatyuk, A.v.
AU - Takacs, Sandor
AU - Capote, R.
N1 - Funding Information:
All co-authors are grateful to the NDS-IAEA for continuously stimulating and effectively supporting their effort in developing and extension of the medical nuclear database. The work described in this paper would not have been possible without assistance in the work of the participating laboratories and the support by IAEA member state contributions.
Publisher Copyright:
© 2023 Elsevier B.V.
PY - 2023/11
Y1 - 2023/11
N2 - Reaction cross sections for production of 11 radionuclides with emerging interest in SPECT imaging are evaluated. Experimental cross section datasets for 40 possible production routes were compiled, discussed and a selection of sets per reaction was proposed for Pade ' fitting leading to recommended values with uncertainties. Only routes for which at least two independent experimental studies were found, with enough data in overlapping energy regions, were considered for selection and fitting. The results of the compilations and available fits are discussed for reactions leading to interesting SPECT radioisotopes: 44mSc (3 routes), 87mY (5 routes), 87gY (m+) (5 routes), 88Y (1 route), 97Ru (5 routes), 131I (1 route), 155Tb (4 routes), 159Gd (3 routes),167Tm-167mEr (8 routes), 191Os-191mIr (2 routes) and 203Pb (2 routes). Integral production yields, based on the Pade ' fits as recommended data, are calculated. A comparison of experimental sets with TALYS-code calculations (results in TENDL-2019 and TENDL-2021 libraries) is made.
AB - Reaction cross sections for production of 11 radionuclides with emerging interest in SPECT imaging are evaluated. Experimental cross section datasets for 40 possible production routes were compiled, discussed and a selection of sets per reaction was proposed for Pade ' fitting leading to recommended values with uncertainties. Only routes for which at least two independent experimental studies were found, with enough data in overlapping energy regions, were considered for selection and fitting. The results of the compilations and available fits are discussed for reactions leading to interesting SPECT radioisotopes: 44mSc (3 routes), 87mY (5 routes), 87gY (m+) (5 routes), 88Y (1 route), 97Ru (5 routes), 131I (1 route), 155Tb (4 routes), 159Gd (3 routes),167Tm-167mEr (8 routes), 191Os-191mIr (2 routes) and 203Pb (2 routes). Integral production yields, based on the Pade ' fits as recommended data, are calculated. A comparison of experimental sets with TALYS-code calculations (results in TENDL-2019 and TENDL-2021 libraries) is made.
KW - PROTON-INDUCED REACTIONSDEUTERON-INDUCED REACTIONSALPHA-INDUCED REACTIONSEXCITATION-FUNCTIONSENERGY-RANGEXN REACTIONSSR-NATNATURAL TITANIUMI-131 SPECTTI-NAT
UR - http://www.scopus.com/inward/record.url?scp=85172867306&partnerID=8YFLogxK
U2 - 10.1016/j.nimb.2023.165119
DO - 10.1016/j.nimb.2023.165119
M3 - Article
VL - 544
SP - 1
EP - 38
JO - Nuclear Instruments and Methods in Physics Research. Section B, Beam Interactions with Materials and Atoms
JF - Nuclear Instruments and Methods in Physics Research. Section B, Beam Interactions with Materials and Atoms
SN - 0168-583X
M1 - 165119
ER -